Diversity in magnetic properties of 3D isomorphous networks of Co(II) and Mn(II) constructed by napthalene-1,4-dicarboxylate.

نویسندگان

  • Tapas Kumar Maji
  • Wakako Kaneko
  • Masaaki Ohba
  • Susumu Kitagawa
چکیده

Two novel 3D isomorphous organic-inorganic hybrid frameworks, [M(1,4-napdc)]n ( M = Co(II), and Mn(II), ; 1,4-napdcH2 = napthalene-1,4-dicarboxylic acid) have been hydrothermally synthesized and structurally characterized, and the magnetic results exhibit metamagnetic behaviour (TC = 5.5 K), and a weak antiferromagnetic interaction, which are structurally correlated.

برای دانلود رایگان متن کامل این مقاله و بیش از 32 میلیون مقاله دیگر ابتدا ثبت نام کنید

ثبت نام

اگر عضو سایت هستید لطفا وارد حساب کاربری خود شوید

منابع مشابه

Novel manganese(II) and cobalt(II) 3D polymers with mixed cyanate and carboxylate bridges: crystal structure and magnetic properties.

Two isomorphous 3D Mn(II) and Co(II) coordination polymers with a dicarboxylate inner salt and cyanate as coligands were synthesized and structurally characterized, and their magnetic properties have been studied. In the compounds, [M(L)(NCO)](n).nH(2)O (M = Mn, Co, L = 1-carboxymethylpyridinium-4-carboxylate), neighboring metal ions are linked by the 3-fold bridges of an end-on cyanate and two...

متن کامل

Two isomorphous Mn(II) and Co(II) 5-amino-tetrazolate coordination polymers with magnetic Δ-chains: crystal structures and magnetic properties.

Two Co(II) and Mn(II) coordination polymers, which have been synthesized under hydrothermal conditions, are isomorphous with magnetic Δ-chains containing trinuclear triangular [M(3)(μ(3)-OH)] clusters. The Δ-chains are bridged by isonicotinic spacers to generate a two-dimensional scalariform layer structure. Magnetic investigations indicate that Co(II) compound exhibits not only spin canting bu...

متن کامل

MOFs constructed with the newly designed imidazole dicarboxylate bearing a 2-position aromatic substituent: hydro(solvo)thermal syntheses, crystal structures and properties.

Six metal-organic frameworks, namely, [Cd(μ(2)-HDMPhIDC)(Py)](n) (H(3)DMPhIDC = 2-(3,4-dimethylphenyl)-1H-imidazole-4,5-dicarboxylic acid, Py = pyridine) (1), [Sr(μ(2)-HDMPhIDC)(H(2)O)](n) (2), {[M1(3)(μ(3)-DMPhIDC)(2)(H(2)O)(6)]·2H(2)O}(n) (M1 = Zn (3), or Mn (4)), [M2(μ(2)-HDMPhIDC)(H(2)O)(2)](n) (M2 = Mg (5), or Ca (6)), have been hydro(solvo)thermally synthesized and structurally characteri...

متن کامل

Structures and magnetic properties of copper(II) and manganese(II) polymers derived from pseudohalides and a flexible zwitterionic dicarboxylate ligand.

The flexible zwitterionic dicarboxylate ligand 1,4-bis(4-carboxylato-1-pyridinium)butane (bcpb) assumes different conformations to collaborate with pseudohalides in various coordination modes to produce coordination polymers in which distinct anionic motifs with mixed carboxylate and pseudohalide bridges are interlinked by the cationic butylenebis(pyridinium) tethers. The Cu(II) compound, [Cu2(...

متن کامل

Manganese(II) pyrimidine-4,6-dicarboxylates: synthetic, structural, magnetic, and adsorption insights.

A series of manganese(II) coordination polymers containing the bridging ligand pyrimidine-4,6-dicarboxylate (pmdc) have been prepared. The stoichiometries and structural features of these materials, which range from the one-dimensional (1D) chains in ([Mn(mu-pmdc)(H2O)3].2H2O)n (1) and ([Mn2(mu-pmdc)2(H2O)5].2H2O)n (2) to the two-dimensional layers in ([Mn(mu3-pmdc)(H2O)].H2O)n (3) or the three...

متن کامل

ذخیره در منابع من


  با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید

عنوان ژورنال:
  • Chemical communications

دوره 36  شماره 

صفحات  -

تاریخ انتشار 2005